Chiral Amphiphilic Au23 Cluster and Its Specific Recognition to Remote Di‐amines
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| Publicado en: | Chemistry vol. 30, no. 65 (Nov 2024) |
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| 022 | |a 0947-6539 | ||
| 022 | |a 1521-3765 | ||
| 024 | 7 | |a 10.1002/chem.202403034 |2 doi | |
| 035 | |a 3131312079 | ||
| 045 | 2 | |b d20241101 |b d20241130 | |
| 084 | |a 162536 |2 nlm | ||
| 100 | 1 | |a Wu, Junfei |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 245 | 1 | |a Chiral Amphiphilic Au<sub>23</sub> Cluster and Its Specific Recognition to Remote Di‐amines | |
| 260 | |b Wiley Subscription Services, Inc. |c Nov 2024 | ||
| 513 | |a Journal Article | ||
| 520 | 3 | |a The atomic precision of metal nanoclusters and variability of surface ligands pave the way for their rational design and functionalization, whereas the property strengthening in multiple ways has been long challenging. Herein, improved amphiphilicity, chirality, thermostability, and strong CPL (circularly polarized luminescence) properties have been accomplished by facile ligand exchange of [Au23(CHT)16]− with HCapt (HCHT and HCapt denote cyclohexanethiol and captopril). In addition, the obtained chiral [Au23(SR)16]− (short for [Au23(CHT)16‐x(Capt)x]−) clusters show specific binding affinity to remote‐diamines (such as arginine and single/double strand DNA), originating from the hydrogen bonding and Van der Waals interaction among the surface Capt ligands and the di‐amine groups. | |
| 653 | |a Diamines | ||
| 653 | |a Thermal stability | ||
| 653 | |a Circular polarization | ||
| 653 | |a Amines | ||
| 653 | |a Cyclohexanethiol | ||
| 653 | |a Ligands | ||
| 653 | |a Captopril | ||
| 653 | |a Nanoclusters | ||
| 653 | |a Hydrogen bonding | ||
| 653 | |a Chirality | ||
| 700 | 1 | |a Wang, Chen |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Chen, Ling |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Lv, Ying |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Cui, Mengting |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Li, Qingliang |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Zhang, Xiangyu |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Yu, Haizhu |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 700 | 1 | |a Zhu, Manzhou |u Department of Chemistry and Centre for Atomic Engineering of Advanced Materials, Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials, Key Laboratory of Structure and Functional Regulation of Hybrid Materials (Anhui University), Ministry of Education, Hefei, Anhui, P. R. China | |
| 773 | 0 | |t Chemistry |g vol. 30, no. 65 (Nov 2024) | |
| 786 | 0 | |d ProQuest |t Health & Medical Collection | |
| 856 | 4 | 1 | |3 Citation/Abstract |u https://www.proquest.com/docview/3131312079/abstract/embedded/7BTGNMKEMPT1V9Z2?source=fedsrch |