Mercapto-functionalized siloxane for enhanced conservation of tremolite jade artifacts

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Publicado en:Heritage Science vol. 13, no. 1 (Dec 2025), p. 212
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Springer Nature B.V.
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Acceso en línea:Citation/Abstract
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022 |a 2050-7445 
024 7 |a 10.1038/s40494-025-01752-5  |2 doi 
035 |a 3208032803 
045 2 |b d20251201  |b d20251231 
084 |a 243040  |2 nlm 
245 1 |a Mercapto-functionalized siloxane for enhanced conservation of tremolite jade artifacts 
260 |b Springer Nature B.V.  |c Dec 2025 
513 |a Journal Article 
520 3 |a Numerous tremolite jade artifacts from archaeological sites exhibit powdering damage, necessitating immediate consolidation. However, research on jade consolidants remains limited. Siloxane is a promising material, yet its effectiveness is hindered by high levels of non-silicate components, such as calcium and magnesium, in tremolite. In this study, mercapto-functionalized siloxane sols with varying mercapto group contents were synthesized via sol–gel chemistry using (3-mercaptopropyl) trimethoxysilane (MPTS), (3-aminopropyl) dimethoxymethylsilane (APDMOS), and tetraethoxysilane (TEOS). Their consolidation effects on tremolite jade were evaluated. Results showed that mercapto-functionalized siloxane exhibited stronger performance than non-functionalized siloxane. This improvement stems from its dual functionality: alkoxy groups undergo hydrolysis and polycondensation to form highly polymerized xerogels that fill microvoids, while thiol groups (–SH) coordinate with calcium and magnesium ions in tremolite, acting as a functional “glue” to bind particles. Mercapto-functionalization thus offers a promising strategy to optimize jade consolidation and improve compatibility with non-silicate substrates. 
653 |a Xerogels 
653 |a Magnesium 
653 |a Sol-gel processes 
653 |a Tetraethyl orthosilicate 
653 |a Powdering 
653 |a Artifacts 
653 |a Chemical synthesis 
653 |a Historic sites 
653 |a Consolidation 
653 |a Tremolite 
653 |a Calcium 
653 |a Siloxanes 
653 |a Nuclear magnetic resonance--NMR 
653 |a Laboratories 
653 |a Chinese history 
653 |a Silica 
653 |a Historic buildings & sites 
653 |a Molecular structure 
653 |a Performance evaluation 
653 |a Physical properties 
653 |a Contact angle 
653 |a Cultural heritage 
773 0 |t Heritage Science  |g vol. 13, no. 1 (Dec 2025), p. 212 
786 0 |d ProQuest  |t Materials Science Database 
856 4 1 |3 Citation/Abstract  |u https://www.proquest.com/docview/3208032803/abstract/embedded/CH9WPLCLQHQD1J4S?source=fedsrch 
856 4 0 |3 Full Text - PDF  |u https://www.proquest.com/docview/3208032803/fulltextPDF/embedded/CH9WPLCLQHQD1J4S?source=fedsrch