Validation and uncertainty estimation for multielement determination using ICP-OES according to the ASTM E2941-14 standard

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Publicat a:Journal of Chemical Metrology vol. 19, no. 1 (Jan-Jun 2025), p. 22-44
Autor principal: Martínez-Peñuñuri, Rodrigo
Altres autors: Alejandro Monserrat GarcÍa Alegria, Vázquez-Bustamante, Paulina, Montoya-Blumenkron, Marcela, Estrada-Gonzalez, Dayana Itzajara, Avilés Figueroa, Ana María, Quizan-Plata, Trinidad, Karla Denisse Murillo-Castillo
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ACG Publications
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022 |a 1307-6183 
024 7 |a 10.25135/jcm.112.2502.3435  |2 doi 
035 |a 3227030971 
045 2 |b d20250101  |b d20250630 
084 |a 277330  |2 nlm 
100 1 |a Martínez-Peñuñuri, Rodrigo 
245 1 |a Validation and uncertainty estimation for multielement determination using ICP-OES according to the ASTM E2941-14 standard 
260 |b ACG Publications  |c Jan-Jun 2025 
513 |a Journal Article 
520 3 |a Standardized analytical methods for determining elemental concentrations require thorough validation and estimation of measurement uncertainty. Inductively coupled plasma optical emission spectrometry (ICP-OES) is a widely used technique for multielement analysis with the ASTM E2941-14 standard specifying the analytical conditions for its application. This study aims to validate the ICP-OES method and estimate the expanded uncertainty for multielement determination in accordance with ASTM E2941-14. Method validation and uncertainty estimation were conducted following Eurachem (2014) and Eurachem-CITAC (2012) guidelines, respectively. The method demonstrated acceptable linearity, with coefficients of determination (R2) ranging from 0.9972 to 1.0000 and correlation coefficients (R) from 0.9982 to 1.0000, exceeding the acceptance criterion (R2/R ≥ 0.995). Accuracy under repeatability conditions showed coefficients of variation between 1.0% and 8.0%, indicating good consistency. Trueness evaluation revealed no significant bias, with recovery rates within the acceptable range of 100% ± 10%. Combined uncertainty values ranged from 0.0425 (silver; Ag) to 0.5156 (scandium; Sc), corresponding to relative uncertainties of 1.25% to 8.16%, respectively. Expanded uncertainties ranged from 0.0850 (Ag) to 1.0312 (Sc). The dominant sources of relative uncertainty were associated with calibration curve-based concentration measurements and volumetric equipment. 
653 |a Quality standards 
653 |a Accuracy 
653 |a Scientific imaging 
653 |a Reference materials 
653 |a Chemical elements 
653 |a Accreditation 
653 |a Calibration 
653 |a Hydrochloric acid 
653 |a Quality control 
653 |a Accountability 
653 |a Laboratories 
700 1 |a Alejandro Monserrat GarcÍa Alegria 
700 1 |a Vázquez-Bustamante, Paulina 
700 1 |a Montoya-Blumenkron, Marcela 
700 1 |a Estrada-Gonzalez, Dayana Itzajara 
700 1 |a Avilés Figueroa, Ana María 
700 1 |a Quizan-Plata, Trinidad 
700 1 |a Karla Denisse Murillo-Castillo 
773 0 |t Journal of Chemical Metrology  |g vol. 19, no. 1 (Jan-Jun 2025), p. 22-44 
786 0 |d ProQuest  |t Biological Science Database 
856 4 1 |3 Citation/Abstract  |u https://www.proquest.com/docview/3227030971/abstract/embedded/6A8EOT78XXH2IG52?source=fedsrch 
856 4 0 |3 Full Text - PDF  |u https://www.proquest.com/docview/3227030971/fulltextPDF/embedded/6A8EOT78XXH2IG52?source=fedsrch