Kinetic behaviour of the roasting/selective reduction process with the use of a mixture of bituminous coal and fuel oil as the additive

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Publicado en:Hemijska Industrija vol. 79, no. 2 (2025), p. 69-79
Autor principal: Angulo-Palma, Hugo Javier
Otros Autores: Saldana, Manuel, Legrá, Legrá Ángel, Urgellés, Alisa Lamorú, Pedrera Carlos Hernández, Gallegos, Sandra, Galleguillos Madrid Felipe M., Toro, Norman
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Hemijska Industrija
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022 |a 0367-598X 
022 |a 2217-7426 
024 7 |a 10.2298/HEMIND240918005A  |2 doi 
035 |a 3241515358 
045 2 |b d20250401  |b d20250630 
100 1 |a Angulo-Palma, Hugo Javier 
245 1 |a Kinetic behaviour of the roasting/selective reduction process with the use of a mixture of bituminous coal and fuel oil as the additive 
260 |b Hemijska Industrija  |c 2025 
513 |a Journal Article 
520 3 |a Lateritic ore is currently the main raw material that allows extraction of Ni by the Caron process. To date, the kinetic behaviour of the roasting/selective reduction process of lateritic nickeli-ferous ores on a pilot scale is largely unknown. In the present study, the kinetic behaviour, the controlling stage and the mechanisms that describe this process with the use of a mixture of 2 wt.% bituminous coal and 1.25 wt.% fuel oil as a reducing additive were determined during the evaluation of the high and low thermal profiles, respectively. The phases of the reduced/le-ached minerals and the fed ore were analysed by X-ray powder diffraction. It was observed that the mixture used as a reducing additive guarantees an adequate transformation in both thermal profiles; the relationship between the residual Ni and residence time is described by a first-order reaction with the determination coefficients greater than 0.949. Although the influence of post-combustion air is not analysed, the controlling stage was diffusion through the ash layer with an activation energy of 14.4060 kJ mol-1. Thus, the most precise combination to describe the process is diffusion through the ash layer and the growth of the nuclei. 
653 |a Thermal transformations 
653 |a X ray powder diffraction 
653 |a Fuel oils 
653 |a Diffusion layers 
653 |a Bituminous coal 
653 |a Raw materials 
653 |a Mixtures 
653 |a Ashes 
653 |a Roasting 
653 |a Furnaces 
653 |a Minerals 
653 |a Chemical elements 
653 |a Temperature 
653 |a Particle size 
653 |a Nickel 
653 |a Coal 
700 1 |a Saldana, Manuel 
700 1 |a Legrá, Legrá Ángel 
700 1 |a Urgellés, Alisa Lamorú 
700 1 |a Pedrera Carlos Hernández 
700 1 |a Gallegos, Sandra 
700 1 |a Galleguillos Madrid Felipe M. 
700 1 |a Toro, Norman 
773 0 |t Hemijska Industrija  |g vol. 79, no. 2 (2025), p. 69-79 
786 0 |d ProQuest  |t Engineering Database 
856 4 1 |3 Citation/Abstract  |u https://www.proquest.com/docview/3241515358/abstract/embedded/7BTGNMKEMPT1V9Z2?source=fedsrch 
856 4 0 |3 Full Text - PDF  |u https://www.proquest.com/docview/3241515358/fulltextPDF/embedded/7BTGNMKEMPT1V9Z2?source=fedsrch