Impact of NVP Doping on the Holographic Properties of PQ/PMMA Holographic Storage Materials

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Publicado en:Polymers vol. 17, no. 17 (2025), p. 2321-2338
Autor principal: Lin, Peng
Otros Autores: Wu, Junhui, Zheng Shujun, Liu, Hongjie, Xiong Ruying, Chen, Xueyan, Xu, Zheng, Lin, Xiao, Tan, Xiaodi
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024 7 |a 10.3390/polym17172321  |2 doi 
035 |a 3249713267 
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100 1 |a Lin, Peng  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
245 1 |a Impact of NVP Doping on the Holographic Properties of PQ/PMMA Holographic Storage Materials 
260 |b MDPI AG  |c 2025 
513 |a Journal Article 
520 3 |a Photopolymer PQ/PMMA, as a pivotal material in the field of holographic storage, demonstrates significant application potential owing to its advantages, such as straightforward preparation processes, cost-effectiveness, and tunable thickness. However, its practical application is still constrained by the need for further enhancement in key performance indicators, including diffraction efficiency, photosensitivity, and anti-aging properties. In this study, N-vinylpyrrolidone (NVP) is employed as a comonomer. By precisely controlling the doping ratio, we systematically investigate the influence mechanism of different NVP doping concentrations on the holographic performance of NVP-PQ/PMMA materials. Research indicates that the introduction of NVP effectively increases the vinyl concentration in the PQ/PMMA matrix, thereby directly generating photoproducts with PQ during the photoreaction process and further enhancing the photopolymerization process. Consequently, the holographic performance of the novel NVP-PQ/PMMA material is improved in a multi-faceted manner compared to ordinary PQ/PMMA. Specifically, the diffraction efficiency is enhanced by 1.93 times, the photosensitivity is increased by 1.64 times, the material uniformity is improved by 38%, and the light-induced shrinkage rate is reduced by 39%. Additionally, NVP-PQ/PMMA materials exhibit excellent stability and aging resistance in high-temperature accelerated aging experiments. Doping with a monomer of specific structure enhances the optical properties, providing broad adaptability for further research on PQ/PMMA photopolymer materials. 
651 4 |a Shanghai China 
651 4 |a China 
653 |a Polymers 
653 |a Photosensitivity 
653 |a Doping 
653 |a Photopolymers 
653 |a Holography 
653 |a Aging 
653 |a Photopolymerization 
653 |a Polymerization 
653 |a Optical properties 
653 |a Polymethyl methacrylate 
653 |a Molecular structure 
653 |a High temperature 
653 |a Aging (materials) 
653 |a Diffraction efficiency 
653 |a Cost effectiveness 
653 |a Efficiency 
653 |a Diffraction 
653 |a Business metrics 
700 1 |a Wu, Junhui  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
700 1 |a Zheng Shujun  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
700 1 |a Liu, Hongjie  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
700 1 |a Xiong Ruying  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
700 1 |a Chen, Xueyan  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
700 1 |a Xu, Zheng  |u College of Photonic and Electronic Engineering, Fujian Normal University, Fuzhou 350117, China; pllsia@163.com (L.P.); junhuifjnu@foxmail.com (J.W.); qbx20240120@yjs.fjnu.edu.cn (S.Z.); qbx20220092@yjs.fjnu.edu.cn (H.L.); xiongruying0217@163.com (R.X.); 15980196902@163.com (X.C.); 15583687780@163.com (X.Z.) 
700 1 |a Lin, Xiao  |u Information Photonics Research Center, Key Laboratory of Optoelectronic Science and for Medicine of Ministry of Education, Fujian Provincial Key Laboratory of Photonics Technology, Fujian Provincial Engineering Technology Research Center of Photoelectric Sensing Application, Fujian Normal University, Fuzhou 350117, China 
700 1 |a Tan, Xiaodi  |u Information Photonics Research Center, Key Laboratory of Optoelectronic Science and for Medicine of Ministry of Education, Fujian Provincial Key Laboratory of Photonics Technology, Fujian Provincial Engineering Technology Research Center of Photoelectric Sensing Application, Fujian Normal University, Fuzhou 350117, China 
773 0 |t Polymers  |g vol. 17, no. 17 (2025), p. 2321-2338 
786 0 |d ProQuest  |t Materials Science Database 
856 4 1 |3 Citation/Abstract  |u https://www.proquest.com/docview/3249713267/abstract/embedded/7BTGNMKEMPT1V9Z2?source=fedsrch 
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